Browsing by Author "Baek, J. H."
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Item Open Access Dislocation density dependent electroabsorption in epitaxial lateral overgrown InGaN/GaN quantum structures(Optical Society of America, 2013-01-14) Sari, E.; Jang, L. W.; Baek, J. H.; Lee, I. H.; Sun, X. W.; Demir, Hilmi VolkanWe study electroabsorption (EA) behavior of InGaN/GaN quantum structures grown using epitaxial lateral overgrowth (ELOG) in correlation with their dislocation density levels and in comparison to steady state and time-resolved photoluminescence measurements. The results reveal that ELOG structures with decreasing mask stripe widths exhibit stronger EA performance, with a maximum EA enhancement factor of 4.8 compared to the reference without ELOG. The analyses show that the EA performance follows similar trends with decreasing dislocation density as the essential parameters of the photoluminescence spectra (peak position, width and intensity) together with the photoluminescence lifetimes. While keeping the growth window widths constant, compared to photoluminescence behavior, however, EA surprisingly exhibits the largest performance variation, making EA the most sensitive to the mask stripe widths. (C) 2013 Optical Society of AmericaItem Open Access Electric field dependent radiative decay kinetics of polar InGaN/GaN quantum heterostructures at low fields(American Institute of Physics, 2009-05-29) Sari, E.; Nizamoglu, S.; Lee, I. H.; Baek, J. H.; Demir, Hilmi VolkanElectric field dependent photoluminescence decay kinetics and its radiative component are studied in polar InGaN/GaN quantum heterostructures at low fields. Under externally applied electric field lower than polarization fields, spectrally and time resolved photoluminescence measurements are taken to retrieve internal quantum efficiencies and carrier lifetimes as a function of the applied field. Subsequently, relative behavior of radiative recombination lifetimes is obtained in response to the applied field. In these characterizations of polar InGaN/GaN structures, we observe that both the carrier lifetime and the radiative recombination lifetime decrease with increasing external electric field, with the radiative component exhibiting weaker field dependence.Item Open Access Experimental and computational analyses of electroabsorption in polar InGaN/GaN quantum zigzag heterostructures(IEEE, 2008-11) Sarı, Emre; Özel, Tuncay; Koç, Aslı; Ju, J.-W.; Ahn, H.-K.; Lee, I.-H.; Baek, J. H.; Demir, Hilmi VolkanTraditional quantum confined Stark effect is well known to lead to strong electroabsorption in multiple quantum well (MQW) structures, yielding only red-shift of the absorption edge with the externally applied electric field, independent of the direction of the applied field. However, a little is known the electroabsorption behavior in III nitride quantum structures grown on c-plane of their wurtzite crystal structure, which is substantially different than the electroabsorption of conventional quantum structures. Such III-N heterostructures exhibit strong polarization fields and discontinuity of such polarization fields at their heterointerfaces causes stimulation of large electrostatic fields in alternating directions for their wells and barriers. Consequently, their energy band diagrams form a zigzag potential profile in conduction and valence bands, instead of those with square profiles. A natural and suitable approach for understanding these polarization fields and also developing insight to design related devices (e.g., electroabsorption modulators) is to study electroabsorption behavior as a function of the polarization field in such polar structures. To this end, we present a comparative, computational and experimental study of electroabsorption in our different designs of c-plane grown polar InGaN/GaN quantum structures with varying levels of polarization.Item Open Access FRET-LEDs involving colloidal quantum dot nanophosphors(Webcom Communications, 2010) Nizamoğlu, S.; Sari, E.; Baek, J. H.; Lee, I. H.; Sun, X. W.; Demir, Hilmi VolkanSemiconductor nanocrystal quantum dots (NQD) with their narrow and tuneable emission are promising candidates to serve as color convertors integrated on light-emitting diodes (LEDs). The use of nonradiative energy transfer, also known as Förster-type resonance energy transfer (FRET), in such NQD nanophosphors provides additional benefits for color-conversion in solid state lighting. In this paper we discuss these NQD-integrated FRET-LEDs for lighting applications.Item Open Access Green/yellow solid state lighting via radiative and nonradiative energy transfer involving colloidal semiconductor nanocrystals(IEEE, 2009-08-05) Nizamoglu, S.; Sari, E.; Baek, J. H.; Lee, I. H; Demir, Hilmi VolkanLEDs made of In(x)Ga(1-x)N and (Al(x)Ga(1-x))(1-y)In(y)P suffer from significantly reduced quantum efficiency and luminous efficiency in the green/yellow spectral ranges. To address these problems, we present the design, growth, fabrication, hybridization, and characterization of proof-of-concept green/yellow hybrid LEDs that utilize radiative and nonradiative [Forster resonance energy transfer (FRET)] energy transfers in their colloidal semiconductor nanocrystals (NCs) integrated on near-UV LEDs. In our first NC-LED, we realize a color-converted LED that incorporate green-emitting CdSe/ZnS core/shell NCs (lambda(PL) = 548 nm) on near-UV InGaN/GaN LEDs (lambda(EL) = 379 nm). In our second NC-LED, we implement a color-converted FRET-enhanced LED. For that, we hybridize a custom-design assembly of cyan-and green-emitting CdSe/ZnS core/shell NCs (lambda(PL) = 490 and 548 nm) on near-UV LEDs. Using a proper mixture of differently sized NCs, we obtain a quantum efficiency enhancement of 9% by recycling trapped excitons via FRET. With FRET-NC-LEDs, we show that it is possible to obtain a luminous efficacy of 425 lm/W(opt) and a luminous efficiency of 94 lm/W, using near-UV LEDs with a 40% external quantum efficiency. Finally, we investigate FRET-converted light-emitting structures that use nonradiative energy transfer directly from epitaxial quantum wells to colloidal NCs. These proof-of-concept demonstrations show that FRET-based NC-LEDs hold promise for efficient solid-state lighting in green/yellow.Item Open Access Nonradiative resonance energy transfer directed from colloidal CdSe/ZnS quantum dots to epitaxial InGaN/GaN quantum wells for solar cells(Wiley, 2010-06-04) Nizamoglu, S.; Sari, E.; Baek, J. H.; Lee, I. H.; Demir, Hilmi VolkanWe report on Förster-type nonradiative resonance energy transfer (NRET) directed from colloidal quantum dots (QDs) to epitaxial quantum wells (QWs) with an efficiency of 69.6% at a rate of 1.527 ns-1 for potential application in III-nitride based photovoltaics. This hybrid exciton generation-collection system consists of chemically-synthesized cyan CdSe/ZnS core/shell QDs (λPL = 490 nm) intimately integrated on epitaxially-grown green InGaN/GaN QWs (λPL = 512 nm). To demonstrate directional NRET from donor QDs to acceptor QWs, we simultaneously show the decreased photoluminescence decay lifetime of dots and increased lifetime of wells in the hybrid dipole-dipole coupled system.Item Open Access Opposite carrier dynamics and optical absorption characteristics under external electric field in nonpolar vs. polar InGaN/GaN based quantum heterostructures(Optical Society of America, 2011) Sari, E.; Nizamoglu, S.; Choi, J H.; Lee, S J.; Baik, K H.; Lee, I. H.; Baek, J. H.; Hwang, S M.; Demir, Hilmi VolkanWe report on the electric field dependent carrier dynamics and optical absorption in nonpolar a-plane GaN-based quantum heterostructures grown on r-plane sapphire, which are surprisingly observed to be opposite to those polar ones of the same materials system and similar structure grown on c-plane. Confirmed by their time-resolved photoluminescence measurements and numerical analyses, we show that carrier lifetimes increase with increasing external electric field in nonpolar InGaN/GaN heterostructure epitaxy, whereas exactly the opposite occurs for the polar epitaxy. Moreover, we observe blue-shifting absorption spectra with increasing external electric field as a result of reversed quantum confined Stark effect in these polar structures, while we observe red-shifting absorption spectra with increasing external electric field because of standard quantum confined Stark effect in the nonpolar structures. We explain these opposite behaviors of external electric field dependence with the changing overlap of electron and hole wavefunctions in the context of Fermi's golden rule. (C) 2011 Optical Society of America