Browsing by Subject "Magnetism"

Now showing 1 - 20 of 25

Open Access
The effect of gadolinium doping on the structural, magnetic and photoluminescence properties of electrospun bismuth ferrite nanofibers
(Elsevier Ltd, 2015) George Philip G.; Senthamizhan, A.; Srinivasan Natarajan, T.; Chandrasekaran G.; Annal Therese H.
Gadolinium (Gd) doped Bismuth ferrite (BFO) nanofibers (Bi1-xGdxFeO3 (x=0.0, 0.05, 0.10, 0.15 and 0.20)) were synthesized via electrospinning. Scanning Electron Microscope (SEM) analysis showed that the diameter of the nanofibers ranged from 150 to 250 nm. X-Ray Diffraction (XRD) analysis revealed a structural phase transition with varying 'x', the compositions with x≤0.10 have crystal structures with space group R3c, while the compositions with x > 0.10 have crystal structures with space group Pnma. Vibrating Sample Magnetometer (VSM) analysis exhibited the weak ferromagnetic nature of the BFO nanofibers. However an increase in the saturated magnetic moment with increase in Gd dopant concentration was observed. The Photoluminescence (PL) spectra of the Bi:1-x :x nanofibers show enhanced Near Band Emission (NBE) intensity at x=0.10 due to the passivation of oxygen vacancies by Gd doping. © 2015 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
Open Access
Effect of magnetic field on the radial pulsations of a gas bubble in a non-Newtonian fluid
(Elsevier Ltd, 2015) Behnia, S.; Mobadersani F.; Yahyavi, M.; Rezavand, A.; Hoesinpour, N.; Ezzat, A.
Dynamics of acoustically driven bubbles' radial oscillations in viscoelastic fluids are known as complex and uncontrollable phenomenon indicative of highly active nonlinear as well as chaotic behavior. In the present paper, the effect of magnetic fields on the non-linear behavior of bubble growth under the excitation of an acoustic pressure pulse in non-Newtonian fluid domain has been investigated. The constitutive equation [Upper-Convective Maxwell (UCM)] was used for modeling the rheological behaviors of the fluid. Due to the importance of the bubble in the medical applications such as drug, protein or gene delivery, blood is assumed to be the reference fluid. It was found that the magnetic field parameter (B) can be used for controlling the nonlinear radial oscillations of a spherical, acoustically forced gas bubble in nonlinear viscoelastic media. The relevance and importance of this control method to biomedical ultrasound applications were highlighted. We have studied the dynamic behavior of the radial response of the bubble before and after applying the magnetic field using Lyapunov exponent spectra, bifurcation diagrams and time series. A period-doubling bifurcation structure was predicted to occur for certain values of the parameters effects. Results indicated its strong impact on reducing the chaotic radial oscillations to regular ones. © 2015 Elsevier Ltd. All rights reserved.
Open Access
Efficient solution of the combined-field integral equation with the parallel multilevel fast multipole algorithm
(IEEE, 2007-08) Gürel, Levent; Ergül, Özgür
We present fast and accurate solutions of large-scale scattering problems formulated with the combined-field integral equation. Using the multilevel fast multipole algorithm (MLFMA) parallelized on a cluster of computers, we easily solve scattering problems that are discretized with tens of millions of unknowns. For the efficient parallelization of MLFMA, we propose a hierarchical partitioning scheme based on distributing the multilevel tree among the processors with an improved load-balancing. The accuracy of the solutions is demonstrated on scattering problems involving spheres of various radii from 80λ to 110λ. In addition to canonical problems, we also present the solution of real-life problems involving complicated targets with large dimensions. © 2007 IEEE.
Open Access
Electronic structure of conventional slater type antiferromagnetic insulators: AIrO3 (A=Sr, Ba) perovskites
(Institute of Physics, 2022) Koc, Husnu; Mamedov, Amirullah M.; Özbay, Ekmel
The structural, mechanical, and electronic properties of Perovskite BaIrO3 and SrIrO3 compounds based on the density functional theory (DFT) have been examined in four different structures (C2/c, R-3m, P6_3/mmc and Pm-3m) and Pnma structure, respectively. The spin polarized generalized gradient approximation has been used for modeling exchange-correlation effects. As a result of spin polarized calculations, it has been observed that BaIrO3 compound showed magnetic properties in C2/c and R-3m structures, but not in Pm-3m and P6_3/mmc structures. SrIrO3 compound also shows magnetic properties in Pnma structure. The elastic constants have been calculated using the strain-stress method and the other related quantities (the bulk modulus, shear modulus, Young's modulus, Poisson's ratio, anisotropy factor, sound velocities, and Debye temperature) have also been estimated. In electronic band structure calculations, while Pm-3m and P6_3/mmc structures of NaIrO3 compound are metallic and semiconductor (Eg = 1.190 eV indirect), respectively, while C2/c and R-3m structures showing magnetic properties are metallic in spin down state and semiconductor (Eg=0.992 eV indirect and Eg=0.665 eV direct, respectively) in the spin up state. The Pmna structure in the SrIrO3 compound is a semiconductor in both spin states (Eg=0.701 eV “0.632 eV” indirect in the spin up “spin down”). © 2022 Institute of Physics Publishing. All rights reserved.
Open Access
Fabrication and characterization of SmCo5/Nb ferromagnetic/superconducting hybrid thin films grown by RF magnetron sputtering technique
(Elsevier, 2017) Ongun, E.; Kuru, M.; Serhatlıoğlu, M.; Hançer, M.; Ozmetin, A. E.
Ferromagnet/Superconductor (F/S) bilayer hybrids show exclusive states due to the mutual interaction between the superconductor and the underlying ferromagnetic substructures in micron scale. In this work, we aimed to observe the effects of the interaction between superconductivity and magnetism, especially the phenomenon involving the orientation and the size of magnetic stripes has been investigated in a coupled ferromagnetic/superconducting thin-film structure. In the proposed F/S hybrid system by this work, superconducting niobium thin-films were combined with underlying segments of ferromagnetic SmCo5 substructures. 300 nm thick magnetic films fabricated by RF magnetron sputtering techniques were topographically grown in patterns with stripes oriented either transverse to or along the direction of current flow. The elemental and microstructural analyses were conducted by EDX, SEM and GIXRD characterization tools. Low-temperature DC transport measurements were conducted by means of four point probe method in a 9T closed-cycle cryogenic refrigeration system. Transport superconducting properties, transition temperature TC(H) and second critical field HC2(T) were measured in a range of applied magnetic field between H = 0–9 kOe for the hybrid system. The results revealed that the artificial periodic modulation of applied field through preferentially-oriented magnetic stripes could introduce normal and superconducting channels or barriers for the current flow.
Open Access
Fast and accurate solutions of scattering problems involving dielectric objects with moderate and low contrasts
(IEEE, 2007-08) Ergül, Özgür; Gürel, Levent
We consider the solution of electromagnetic scattering problems involving relatively large dielectric objects with moderate and low contrasts. Three-dimensional objects are discretized with Rao-Wilton-Glisson functions and the scattering problems are formulated with surface integral equations. The resulting dense matrix equations are solved iteratively by employing the multilevel fast multipole algorithm. We compare the accuracy and efficiency of the results obtained by employing various integral equations for the formulation of the problem. If the problem size is large, we show that a combined formulation, namely, electric-magnetic current combined-field integral equation, provides faster iterative convergence compared to other formulations, when it is accelerated with an efficient block preconditioner. For low-contrast problems, we introduce various stabilization procedures in order to avoid the numerical breakdown encountered in the conventional surface formulations. © 2007 IEEE.
Open Access
Fourier transform magnetic resonance current density imaging (FT-MRCDI) from one component of magnetic flux density
(IOP Publishing, 2010-05-17) Ider, Y. Z.; Birgul, O.; Oran, O. F.; Arıkan, Orhan; Hamamura, M. J.; Muftuler, L. T.
Fourier transform (FT)-based algorithms for magnetic resonance current density imaging (MRCDI) from one component of magnetic flux density have been developed for 2D and 3D problems. For 2D problems, where current is confined to the xy-plane and z-component of the magnetic flux density is measured also on the xy-plane inside the object, an iterative FT-MRCDI algorithm is developed by which both the current distribution inside the object and the z-component of the magnetic flux density on the xy-plane outside the object are reconstructed. The method is applied to simulated as well as actual data from phantoms. The effect of measurement error on the spatial resolution of the current density reconstruction is also investigated. For 3D objects an iterative FT-based algorithm is developed whereby the projected current is reconstructed on any slice using as data the Laplacian of the z-component of magnetic flux density measured for that slice. In an injected current MRCDI scenario, the current is not divergence free on the boundary of the object. The method developed in this study also handles this situation.
Open Access
Guiding, bending, and splitting of electromagnetic waves in highly confined photonic crystal waveguides
(American Physical Society, 2001) Bayındır, Mehmet; Özbay, Ekmel; Temelkuran, B.; Sigalas, M. M.; Soukoulis, C. M.; Biswas, R.; Ho, K. M.
We have experimentally demonstrated the guiding, bending, and splitting of electromagnetic (EM) waves in highly confined waveguides built around three-dimensional layer-by-layer photonic crystals by removing a single rod. Full transmission of the EM waves was observed for straight and bended waveguides. We also investigated the power splitter structures in which the input EM power could be efficiently divided into the output waveguide ports. The experimental results, dispersion relation and photon lifetime, were analyzed with a theory based on the tight-binding photon picture. Our results provide an important tool for designing photonic crystal based optoelectronic components.
Open Access
High-conducting magnetic nanowires obtained from uniform titanium-covered carbon nanotubes
(American Physical Society, 2004) Daǧ, Sefa; Durgun, Engin; Çıracı, Salim
We have shown that a semiconducting single-wall carbon nanotube (SWNT) can be covered uniformly by titanium atoms and form a complex but regular atomic structure. The circular cross section changes to a squarelike form, and the system becomes metallic with high state density at the Fermi level and with high quantum ballistic conductance. Metallicity is induced not only by the metal-metal coupling, but also by the band-gap closing of SWNT's at the corners of the square. Even more interesting is that uniform titanium-covered tubes have magnetic ground state with significant net magnetic moment. Our results have been obtained by the first-principles pseudopotential plane-wave calculations within the density-functional theory.
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Highly monodisperse low-magnetization magnetite nanocubes as simultaneous T1–T2 MRI contrast agents
(Royal Society of Chemistry, 2015) Sharma, V. K.; Alipour, A.; Soran-Erdem, Z.; Aykut, Z. G.; Demir, Hilmi Volkan
We report the first study of highly monodisperse and crystalline iron oxide nanocubes with sub-nm controlled size distribution (9.7 ± 0.5 nm in size) that achieve simultaneous contrast enhancement in both T1- and T2-weighted magnetic resonance imaging (MRI). Here, we confirmed the magnetite structure of iron oxide nanocubes by X-ray diffraction (XRD), selected area electron diffraction (SAED) pattern, optical absorption and Fourier transformed infrared (FT-IR) spectra. These magnetite nanocubes exhibit superparamagnetic and paramagnetic behavior simultaneously by virtue of their finely controlled shape and size. The magnetic measurements reveal that the magnetic moment values are favorably much lower because of the small size and cubic shape of the nanoparticles, which results in an enhanced spin canting effect. As a proof-of-concept demonstration, we showed their potential as dual contrast agents for both T1- and T2-weighted MRI via phantom studies, in vivo imaging and relaxivity measurements. Therefore, these low-magnetization magnetite nanocubes, while being non-toxic and bio-compatible, hold great promise as excellent dual-mode T1 and T2 contrast agents for MRI. © 2014 The Royal Society of Chemistry.
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Image reconstruction for Magnetic Particle Imaging using an Augmented Lagrangian Method
(IEEE, 2017) Ilbey S.; Top C.B.; Çukur, Tolga; Sarıtaş, Emine Ülkü; Guven H.E.
Magnetic particle imaging (MPI) is a relatively new imaging modality that images the spatial distribution of superparamagnetic iron oxide nanoparticles administered to the body. In this study, we use a new method based on Alternating Direction Method of Multipliers (a subset of Augmented Lagrangian Methods, ADMM) with total variation and l1 norm minimization, to reconstruct MPI images. We demonstrate this method on data simulated for a field free line MPI system, and compare its performance against the conventional Algebraic Reconstruction Technique. The ADMM improves image quality as indicated by a higher structural similarity, for low signal-to-noise ratio datasets, and it significantly reduces computation time. © 2017 IEEE.
Open Access
Magnetic ground state in FeTe2,VS2, and NiTe2 monolayers: antiparallel magnetic moments at chalcogen atoms
(American Physical Society, 2020) Aras, M.; Kılıç, Ç.; Çıracı, Salim
Our analysis based on the results of hybrid and semilocal density-functional calculations with and without Hubbard U correction for on-site Coulomb interactions reveals the true magnetic ground states of three transition-metal dichalcogenide monolayers, viz., FeTe2,VS2, and NiTe2, which comprise inhomogeneous magnetic moment configurations. In contrast to earlier studies considering only the magnetic moments of transition-metal atoms, the chalcogen atoms by themselves have significant, antiparallel magnetic moments owing to the spin polarization through p−d hybridization. The latter is found to be true for both H and T phases of FeTe2,VS2, and NiTe2 monolayers. Our predictions show that the FeTe2 monolayer in its lowest-energy structure is a half metal, which prevails under both compressive and tensile strains. Half metallicity occurs also in the FeTe2 bilayer but disappears in thicker multilayers. The VS2 monolayer is a magnetic semiconductor; it has two different band gaps of different character and widths for different spin polarization. The NiTe2 monolayer, which used to be known as a nonmagnetic metal, is indeed a magnetic metal with a small magnetic moment. These monolayers with intriguing electronic and magnetic properties can attain new functionalities for spintronic applications.
Open Access
Magnetic resonance imaging assisted by wireless passive implantable fiducial e-markers
(Institute of Electrical and Electronics Engineers, 2017) Gokyar, S.; Alipour, A.; Unal, E.; Atalar, Ergin; Demir, Hilmi Volkan
This paper reports a wireless passive resonator architecture that is used as a fiducial electronic marker (e-marker) intended for internal marking purposes in magnetic resonance imaging (MRI). As a proof-of-concept demonstration, a class of double-layer, sub-cm helical resonators were microfabricated and tuned to the operating frequency of 123 MHz for a three T MRI system. Effects of various geometrical parameters on the resonance frequency of the e-marker were studied, and the resulting specific absorption rate (SAR) increase was analyzed using a full-wave microwave solver. The B1 + field distribution was calculated, and experimental results were compared. As an exemplary application to locate subdural electrodes, these markers were paired with subdural electrodes. It was shown that such sub-cm self-resonant e-markers with biocompatible constituents can be designed and used for implant marking, with sub-mm positioning accuracy, in MRI. In this application, a free-space quality factor ( Q -factor) of approximately 50 was achieved for the proposed resonator architecture. However, this structure caused an SAR increase in certain cases, which limits its usage for in vivo imaging practices. The findings indicate that these implantable resonators hold great promise for wireless fiducial e-marking in MRI as an alternative to multimodal imaging.
Open Access
Memory-efficient multilevel physical optics algorithm for fast computation of scattering from three-dimensional complex targets
(IEEE, 2007) Manyas, Alp; Gürel, Levent
Multilevel physical optics (MLPO) algorithm provides a speed-up for computing the physical-optics integral over complex bodies for a range of aspect angles and frequencies. On the other hand, when computation of the RCS pattern as a function of θ, φ, and frequency is desired, the O N3 memory complexity of the algorithm may prevent the solution of electrically large problems. In this paper, we propose an improved version of the MLPO algorithm, for which the memory complexity is reduced to O N2 log N . The algorithm is based on the aggregation of only some portion of the scattering patterns at each aggregation step. This way, memory growth in each step is prevented, and a significant amount of saving is achieved.
Open Access
MLFMA solutions of transmission problems Involving realistic metamaterial walls
(IEEE, 2007-08) Ergül, Özgür; Ünal, Alper; Gürel, Levent
We present the solution of multilayer metamaterial (MM) structures containing large numbers of unit cells, such as split-ring resonators. Integral-equation formulations of scattering problems are solved iteratively by employing a parallel implementation of the multilevel fast multipole algorithm. Due to ill-conditioned nature of the problems, advanced preconditioning techniques are used to obtain rapid convergence in the iterative solutions. By constructing a sophisticated simulation environment, we accurately and efficiently investigate large and complicated MM structures. © 2007 IEEE.
Open Access
Mn2+-doped CdSe/CdS core/multishell colloidal quantum wells enabling tunable carrier-dopant exchange interactions
(American Chemical Society, 2015) Delikanlı, S.; Akgül, M. Z.; Murphy, J. R.; Barman, B.; Tsai, Y.; Scrace, T.; Zhang, P.; Bozok, B.; Hernández-Martínez, P.L.; Christodoulides, J.; Cartwright, A. N.; Petrou, A.; Demir, Hilmi Volkan
In this work, we report the manifestations of carrier-dopant exchange interactions in colloidal Mn2+-doped CdSe/CdS core/multishell quantum wells. The carrier-magnetic ion exchange interaction effects are tunable through wave function engineering. In our quantum well heterostructures, manganese was incorporated by growing a Cd0.985Mn0.015S monolayer shell on undoped CdSe nanoplatelets using the colloidal atomic layer deposition technique. Unlike previously synthesized Mn2+-doped colloidal nanostructures, the location of the Mn ions was controlled with atomic layer precision in our heterostructures. This is realized by controlling the spatial overlap between the carrier wave functions with the manganese ions by adjusting the location, composition, and number of the CdSe, Cd1-xMnxS, and CdS layers. The photoluminescence quantum yield of our magnetic heterostructures was found to be as high as 20% at room temperature with a narrow photoluminescence bandwidth of ∼22 nm. Our colloidal quantum wells, which exhibit magneto-optical properties analogous to those of epitaxially grown quantum wells, offer new opportunities for solution-processed spin-based semiconductor devices. © 2015 American Chemical Society.
Open Access
Orbital magnetization of single and double quantum dots in a tight-binding model
(American Physical Society, 2003) Aldea, A.; Moldoveanu, V.; Niţǎ, M.; Manolescu, A.; Gudmundsson, V.; Tanatar, Bilal
We calculate the orbital magnetization of single and double quantum dots coupled both by Coulomb interaction and by electron tunneling. The electronic states of the quantum dots are calculated in a tight-binding model, and the magnetization is discussed in relation to the energy spectrum and to the edge and bulk states. We identify effects of chirality of the electronic orbits and of the anticrossing of the energy levels when the magnetic field is varied. We also consider the effects of detuning the energy spectra of the quantum dots by an external gate potential. We compare our results with the recent experiments of Oosterkamp et al. [Phys, Rev. Lett. 80, 4951 (1998)].
Open Access
Oxygen partial pressure dependence of magnetic, optical and magneto-optical properties of epitaxial cobalt-substituted SrTiO3 films
(OSA - The Optical Society, 2015) Onbaşli, M.C.; Goto, T.; Tang, A.; Pan, A.; Battal, E.; Okyay, Ali Kemal; Dionne G.F.; Ross, C.A.
Cobalt-substituted SrTiO3 films (SrTi0.70Co0.30O3-δ) were grown on SrTiO3 substrates using pulsed laser deposition under oxygen pressures ranging from 1 μTorr to 20 mTorr. The effect of oxygen pressure on structural, magnetic, optical, and magneto-optical properties of the films was investigated. The film grown at 3 μTorr has the highest Faraday rotation (FR) and magnetic saturation moment (Ms). Increasing oxygen pressure during growth reduced Ms, FR and optical absorption in the nearinfrared. This trend is attributed to decreasing Co2+ ion concentration and oxygen vacancy concentration with higher oxygen partial pressure during growth. © 2015 Optical Society of America.
Open Access
Parallel preconditioners for solutions of dense linear systems with tens of millions of unknowns
(2007-11) Malas, Tahir; Ergül, Özgür; Gürel, Levent
We propose novel parallel preconditioning schemes for the iterative solution of integral equation methods. In particular, we try to improve convergence rate of the ill-conditioned linear systems formulated by the electric-field integral equation, which is the only integral-equation formulation for targets having open surfaces. For moderate-size problems, iterative solution of the near-field system enables much faster convergence compared to the widely used sparse approximate inverse preconditioner. For larger systems, we propose an approximation strategy to the multilevel fast multipole algorithm (MLFMA) to be used as a preconditioner. Our numerical experiments reveal that this scheme significantly outperforms other preconditioners. With the combined effort of effective preconditioners and an efficiently parallelized MLFMA, we are able to solve targets with tens of millions of unknowns, which are the largest problems ever reported in computational electromagnetics. ©2007 IEEE.
Open Access
Quantum turnstile operation of single-molecule magnets
(Institute of Physics Publishing, 2015) Moldoveanu, V.; Dinu, I. V.; Tanatar, Bilal; Moca, C. P.
The time-dependent transport through single-molecule magnets coupled to magnetic or non-magnetic electrodes is studied in the framework of the generalized master equation method. We investigate the transient regime induced by the periodic switching of the source and drain contacts. If the electrodes have opposite magnetizations the quantum turnstile operation allows the stepwise writing of intermediate excited states. In turn, the transient currents provide a way to read these states. Within our approach we take into account both the uniaxial and transverse anisotropy. The latter may induce additional quantum tunneling processes which affect the efficiency of the proposed read-and-write scheme. An equally weighted mixture of molecular spin states can be prepared if one of the electrodes is ferromagnetic. © 2015 IOP Publishing Ltd and Deutsche Physikalische Gesellschaft.