Browsing by Author "Ortaç, B."

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Open Access
1018 nm Yb-doped high-power fiber laser pumped by broadband pump sources around 915 nm with output power above 100 W
(OSA - The Optical Society, 2017) Midilli, Y.; Efunbajo, O. B.; Şimşek, B.; Ortaç, B.
We demonstrate a 1018 nm ytterbium-doped all-fiber laser pumped by tunable pump sources operating in the broad absorption spectrum around 915 nm. In the experiment, two different pump diodes were tested to pump over a wide spectrum ranging from 904 to 924 nm by altering the cooling temperature of the pump diodes. Across this so-called pump wavelength regime having a 20 nm wavelength span, the amplified stimulated emission (ASE) suppression of the resulting laser was generally around 35 dB, showing good suppression ratio. Comparisons to the conventional 976 nm-pumped 1018 nm ytterbium-doped fiber laser were also addressed in this study. Finally, we have tested this system for high power experimentation and obtained 67% maximum optical-to-optical efficiency at an approximately 110 W output power level. To the best of our knowledge, this is the first 1018 nm ytterbium-doped all-fiber laser pumped by tunable pump sources around 915 nm reported in detail.
Open Access
Bio-based polymer nanocomposites based on layered silicates having a reactive and renewable intercalant
(Wiley, 2013) Albayrak, O.; Şen, S.; Çaylbox, G.; Ortaç, B.
Soybean oil-based polymer nanocomposites were synthesized from acrylated epoxidized soybean oil (AESO) combined with styrene monomer and montmorillonite (MMT) clay by using in situ free radical polymerization reaction. Special attention was paid to the modification of MMT clay, which was carried out by methacryl-functionalized and quaternized derivative of methyl oleate intercalant. It was synthesized from olive oil triglyceride, as a renewable intercalant. The resultant nanocomposites were characterized by X-ray diffraction (XRD) and transmission electron microscopy (TEM). The effect of increased nanofiller loading in thermal and mechanical properties of the nanocomposites was investigated by thermogravimetric analysis (TGA) and dynamic mechanical analysis (DMA). The nanocomposites exhibited improved thermal and dynamic mechanical properties compared with neat acrylated epoxidized soybean oil based polymer matrix. The desired exfoliated nanocomposite structure was achieved when the OrgMMT loading was 1 and 2 wt % whereas partially exfoliated nanocomposite was obtained in 3 wt % loading. It was found that about 400 and 500% increments in storage modulus at glass transition and rubbery regions, respectively were achieved at 2 wt % clay loading compared to neat polymer matrix while the lowest thermal degradation rate was gained by introducing 3 wt % clay loading. © 2013 Wiley Periodicals, Inc.
Open Access
CO2 laser polishing of conical shaped optical fiber deflectors
(Springer Verlag, 2017-06) Şimşek, E. U.; Şimşek, B.; Ortaç, B.
A novel method for polishing conical shaped optical fiber deflectors by modulated CO2 laser exposure is reported. The conical shaped fiber deflector geometry was first formed with rough mechanical polishing, then it was exposed to modulated CO2 laser operating with wavelength at 10.6 µm to achieve fine polish surfaces. The motivation of this work is to demonstrate that the modulated CO2 laser exposure approach allows a fiber surface roughness at a nanometer scale without modifying the conical shape of the fiber deflector. The average surface roughness of mechanically polished fiber deflectors with 30 and 9 µm lapping films was smoothed down to 20.4 and 4.07 nm, respectively, after CO2 laser polishing process. By combining mechanical and laser polishing techniques, fabrication of conical shaped optical fiber deflectors takes less time and it becomes laborer independent and easy to apply. © 2017, Springer-Verlag Berlin Heidelberg.
Open Access
CO2 laser polishing of microfluidic channels fabricated by femtosecond laser assisted carving
(Institute of Physics Publishing, 2016-10) Serhatlioglu, M.; Ortaç, B.; Elbuken, C.; Bıyıklı, Necmi; Solmaz, M. E.
In this study, we investigate the effects of CO2 laser polishing on microscopic structures fabricated by femtosecond laser assisted carving (FLAC). FLAC is the peripheral laser irradiation of 2.5D structures suitable for low repetition rate lasers and is first used to define the microwell structures in fused silica followed by chemical etching. Subsequently, the bottom surface of patterned microwells is irradiated with a pulsed CO2 laser. The surfaces were characterized using an atomic force microscope (AFM) and scanning electron microscope (SEM) in terms of roughness and high quality optical imaging before and after the CO2 laser treatment. The AFM measurements show that the surface roughness improves more than threefold after CO2 laser polishing, which promises good channel quality for applications that require optical imaging. In order to demonstrate the ability of this method to produce low surface roughness systems, we have fabricated a microfluidic channel. The channel is filled with polystyrene bead-laden fluid and imaged with transmission mode microscopy. The high quality optical images prove CO2 laser processing as a practical method to reduce the surface roughness of microfluidic channels fabricated by femtosecond laser irradiation. We further compared the traditional and laser-based glass micromachining approaches, which includes FLAC followed by the CO2 polishing technique.
Open Access
Compact ultrafast oscillators and high performance ultrafast amplifiers based on ytterbium-doped fibers
(Springer Verlag, 2016) Limpert, J.; Eidam, T.; Baumgartl, M.; Röser, F.; Plötner, M.; Ortaç, B.; Nolte, S.; Tünnermann, A.
This chapter reviews the fundamentals and achievements of ultrashort pulse generation and amplification in ytterbium-doped fibers. Compact and ultrastable passively mode-locked fiber oscillators represent an ideal seed source for high performance femtosecond fiber amplification systems, which have been scaled towards kW-level average power and pulse energies well above the mJ-level. These laser systems will have significant impact in numerous scientific and industrial applications.
Open Access
Effects of laser ablated silver nanoparticles on Lemna minor
(Elsevier, 2014) Üçüncü, E.; Özkan, A. D.; Kurşungöz, C.; Ülger, Z. E.; Ölmez, T. T.; Tekinay, T.; Ortaç, B.; Tunca E.
Open Access
Electrochemically tunable ultrafast optical response of graphene oxide
(A I P Publishing LLC, 2011) Kürüm, U.; Ekiz, O. Ö.; Yaglioglu, H. G.; Elmali, A.; Ürel, M.; Güner, H.; Mızrak, A. K.; Ortaç, B.; Dâna, A.
We demonstrate reversible and irreversible changes in the ultrafast optical response of multilayer graphene oxide thin films upon electrical and optical stimulus. The reversible effects are due to electrochemical modification of graphene oxide, which allows tuning of the optical response by externally applied bias. Increasing the degree of reduction in graphene oxide causes excited state absorption to gradually switch to saturable absorption for shorter probe wavelengths. Spectral and temporal properties as well as the sign of the ultrafast response can be tuned either by changing the applied bias or exposing to high intensity femtosecond pulses. © 2011 American Institute of Physics.
Open Access
Encapsulation of a zinc phthalocyanine derivative in self-assembled peptide nanofibers
(The Royal Society of Chemistry, 2012) Garifullin, R.; Erkal, T. S.; Tekin, S.; Ortaç, B.; Gürek, A. G.; Ahsen, V.; Yaglioglu, H. G.; Elmali, A.; Güler, Mustafa O.
In this article, we demonstrate encapsulation of octakis(hexylthio) zinc phthalocyanine molecules by non-covalent supramolecular organization within self-assembled peptide nanofibers. Peptide nanofibers containing octakis(hexylthio) zinc phthalocyanine molecules were obtained via a straight-forward one-step self-assembly process under aqueous conditions. Nanofiber formation results in the encapsulation and organization of the phthalocyanine molecules, promoting ultrafast intermolecular energy transfer. The morphological, mechanical, spectroscopic and non-linear optical properties of phthalocyanine containing peptide nanofibers were characterized by TEM, SEM, oscillatory rheology, UV-Vis, fluorescence, ultrafast pump-probe and circular dichroism spectroscopy techniques. The ultrafast pump-probe experiments of octakis(hexylthio) zinc phthalocyanine molecules indicated pH controlled non-linear optical characteristics of the encapsulated molecules within self-assembled peptide nanofibers. This method can provide a versatile approach for bottom-up fabrication of supramolecular organic electronic devices. © 2012 The Royal Society of Chemistry.
Open Access
Enhancement in c-Si solar cells using 16 nm InN nanoparticles
(IOP Publishing, 2016-05) Chowdhury, F. I.; Alnuaimi, A.; Alkis, S.; Ortaç, B.; Aktürk, S.; Alevli, M.; Dietz, N.; Okyay, Ali Kemal; Nayfeh, A.
In this work, 16 nm indium nitride (InN) nanoparticles (NPs) are used to increase the performance of thin-film c-Si HIT solar cells. InN NPs were spin-coated on top of an ITO layer of c-Si HIT solar cells. The c-Si HIT cell is a stack of 2 μm p type c-Si, 4–5 nm n type a-Si, 15 nm n+ type a-Si and 80 nm ITO grown on a p+ type Si substrate. On average, short circuit current density (Jsc) increases from 19.64 mA cm−2 to 21.54 mA cm−2 with a relative improvement of 9.67% and efficiency increases from 6.09% to 7.09% with a relative improvement of 16.42% due to the presence of InN NPs. Reflectance and internal/external quantum efficiency (IQE/EQE) of the devices were also measured. Peak EQE was found to increase from 74.1% to 81.3% and peak IQE increased from 93% to 98.6% for InN NPs coated c-Si HIT cells. Lower reflection of light due to light scattering is responsible for performance enhancement between 400–620 nm while downshifted photons are responsible for performance enhancement from 620 nm onwards.
Open Access
Generation of InN nanocrystals in organic solution through laser ablation of high pressure chemical vapor deposition-grown InN thin film
(Springer, 2012-07-27) Alkis, S.; Alevli, M.; Burzhuev, S.; Vural, H. A.; Okyay, Ali Kemal; Ortaç, B.
We report the synthesis of colloidal InN nanocrystals (InN-NCs) in organic solution through nanosecond pulsed laser ablation of high pressure chemical vapor deposition-grown InN thin film on GaN/sapphire template substrate. The size, the structural, the optical, and the chemical characteristics of InN-NCs demonstrate that the colloidal InN crystalline nanostructures in ethanol are synthesized with spherical shape within 5.9-25.3, 5.45-34.8, 3.24-36 nm particle-size distributions, increasing the pulse energy value. The colloidal InN-NCs solutions present strong absorption edge tailoring from NIR region to UV region.
Open Access
Generation of parabolic bound pulses from a Yb-fiber laser
(Optical Society of American (OSA), 2006) Ortaç, B.; Hideur, A.; Brunel, M.; Chédot, C.; Limpert J.; Tünnermann, A.; Ilday F.Ö.
We report the observation of self-similar propagation of bound-state pulses in an ytterbium-doped double-clad fiber laser. A bound state of two positively chirped parabolic pulses with 5.4 ps duration separated by 14.9 ps is obtained, with 1.7 nJ of energy per pulse. These pulses are extra-cavity compressed to 100 fs. For higher pumping power and a different setting of the intra-cavity polarization controllers, the laser generates a bound state of three chirped parabolic pulses with different time separations and more than 1.5 nJ energy per pulse. Perturbation of this bound state by decreasing pump power results in the generation of a single pulse and a two-pulse bound state both structures traveling at the same velocity along the cavity. A possible explanation of the zero relative speed by a particular phase relation of the bound states is discussed. ©2006 Optical Society of America.
Open Access
Generation of ultra-small InN nanocrystals by pulsed laser ablation of suspension in organic solution
(Springer Verlag, 2017-03) Kurşungöz, C.; U. Şimşek, E.; Tuzaklı, R.; Ortaç, B.
Nanostructures of InN have been extensively investigated since nano-size provides a number of advantages allowing applications in nanoscale electronic and optoelectronic devices. It is quite important to obtain pure InN nanocrystals (InN-NCs) to reveal the characteristic features, which gain interest in the literature. Here, we proposed a new approach for the synthesis of ultra-small hexagonal InN-NCs by using suspension of micron-sized InN powder in ethanol with pulsed laser ablation method. The liquid environment, laser energy and ablation time were optimized and a post-synthesis treatment, centrifugation, was performed to achieve InN-NCs with the smallest size. Besides, the micron-sized InN powder suspension, as a starting material, enabled us to obtain InN-NCs having diameters smaller than 5 nm. We also presented a detailed characterization of InN-NCs and demonstrated that the formation mechanism mainly depends on the fragmentation due to laser irradiation of the suspension.
Open Access
Gold nanoparticle / polymer nanofibrous composites by laser ablation and electrospinning
(Elsevier BV, 2011) Deniz, A. E.; Vural, H. A.; Ortaç, B.; Uyar, Tamer
Poly(vinylpyrolidone) (PVP) nanofibers incorporating gold nanoparticles (Au-NPs) were produced in combination with laser ablation and electrospinning techniques. The Au-NPs were directly synthesized in PVP solution by laser ablation and then, the electrospinning of PVP/Au-NPs solution was carried out for obtaining nanofibrous composites. The presence of Au-NPs in the PVP nanofibers was confirmed by SEM, TEM and EDX analyses. The SEM imaging elucidated that the electrospun PVP/Au-NPs nanofibers were bead-free having average fiber diameter of 810 ± 480 nm. The TEM imaging indicated that the Au-NPs were in spherical shape having diameters in the range of 5 to 20 nm and the Au-NPs were more or less dispersed homogeneously in the PVP nanofiber matrix. The FTIR study suggested the presence of molecular interactions between PVP matrix and the Au-NPs in the nanofibrous composites. The UV-Vis measurement confirmed the enhancement of the optical properties of the PVP/Au-NPs nanofibers in the solid state due to the surface plasma resonance effect of Au-NPs. © 2011 Elsevier B.V. All Rights Reserved.
Open Access
High average and peak power femtosecond large-pitch photonic-crystal-fiber laser
(2011) Baumgartl, M.; Jansen F.; Stutzki F.; Jauregui, C.; Ortaç, B.; Limpert J.; Tünnermann, A.
We report on the generation of high-average-power and high-peak-power ultrashort pulses from a mode-locked fiber laser operating in the all-normal-dispersion regime. As gain medium, a large-mode-area ytterbium-doped large-pitch photonic-crystal fiber is used. The self-starting fiber laser delivers 27 W of average power at 50:57 MHz repetition rate, resulting in 534 nJ of pulse energy. The laser produces positively chirped 2 ps output pulses, which are compressed down to sub-100 fs, leading to pulse peak powers as high as 3:2 MW. © 2011 Optical Society of America.
Open Access
High-energy femtosecond photonic crystal fiber laser
(2010) Lecaplain, C.; Ortaç, B.; MacHinet G.; Boullet J.; Baumgart, M.; Schreiber, T.; Cormier, E.; Hideur, A.
We report the generation of high-energy high-peak power pulses in an all-normal dispersion fiber laser featuring large-mode-area photonic crystal fibers. The self-starting chirped-pulse fiber oscillator delivers 11 W of average power at 15:5 MHz repetition rate, resulting in 710 nJ of pulse energy. The output pulses are dechirped outside the cavity from 7 ps to nearly transform-limited duration of 300 fs, leading to pulse peak powers as high as 1:9 MW. Numerical simulations reveal that pulse shaping is dominated by the amplitude modulation and spectral filtering provided by a resonant semiconductor saturable absorber. © 2010 Optical Society of America.
Open Access
Impact of dispersion on pulse dynamics in chirped-pulse fiber lasers
(Springer, 2012-05) Baumgartl, M.; Ortaç, B.; Limpert, J.; Tünnermann, A.
We report on a systematic study of an environmentally stable mode-locked Yb-doped fiber laser operating in the chirped-pulse regime. The linear cavity chirped-pulse fiber laser is constructed with a saturable absorber mirror as nonlinear mode-locking mechanism and a nonlinearity-free transmission-grating-based stretcher/compressor for dispersion management. Mode-locked operation and pulse dynamics from strong normal to strong anomalous total cavity dispersion in the range of +2.5 to -1.6 ps(2) is experimentally studied. Strongly positively chirped pulses from 4.3 ps (0.01 ps(2)) to 39 ps (2.5 ps(2)) are obtained at normal net-cavity dispersion. In the anomalous dispersion regime, the laser generates average soliton feature negatively chirped pulses with autocorrelation pulse durations from 0.8 ps (-0.07 ps(2)) to 3.9 ps (-1.6 ps(2)). The lowered peak power due to the pulse stretching allows one to increase the double pulse threshold. Based on the numerical simulation, different regimes of mode locking are obtained by varying the intra-cavity dispersion, and the characteristics of average soliton, stretched-pulse, wave-breaking-free and chirped-pulse regimes are discussed.
Open Access
Observation of soliton molecules with independently evolving phase in a mode-locked fiber laser
(2010) Ortaç, B.; Zaviyalov, A.; Nielsen, C.K.; Egorov O.; Iliew, R.; Limpert J.; Lederer F.; Tünnermann, A.
We report the experimental generation of two-soliton molecules in an all-polarization-maintaining ytterbium-doped fiber laser operating in the normal dispersion regime. These molecules exhibit an independently evolving phase and are characterized by a regular spectral modulation pattern with a modulation depth of 80% measured as an averaged value. Moreover, the numerical modeling confirms that the limited modulation depth of the spectrum is caused by the evolution of the phase difference between the pulses. © 2010 Optical Society of America.
Open Access
Photoluminescent electrospun polymeric nanofibers incorporating germanium nanocrystals
(Elsevier, 2013) Ortaç, B.; Kayaci, F.; Vural, H. A.; Deniz, A. E.; Uyar, Tamer
The photoluminescent germanium nanocrystals (Ge-NCs) were successfully incorporated into electrospun polymeric nanofiber matrix in order to develop photoluminescent nanofibrous composite web. In the first step, the synthesis of Ge-NCs was achieved by nanosecond pulsed laser ablation of bulk germanium wafer immersed in organic liquid. The size, the structural and the chemical characteristics of Ge-NCs investigated by TEM, XPS, XRD and Raman spectroscopy revealed that the Ge-NCs were highly pure and highly crystalline having spherical shape within 3-20 nm particle size distribution. In the second step, Ge-NCs were mixed with polyvinyl alcohol (PVA) polymer solution, and then, Ge-NC/PVA nanofibers were obtained via electrospinning technique. The electrospinning of Ge-NCs/PVA nanoweb composite structure was successful and bead-free Ge-NCs/PVA nanofibers having average fiber diameter of 185 ± 40 nm were obtained. The STEM analysis of the electrospun Ge-NCs/PVA nanofibers elucidated that the Ge-NCs were distributed homogeneously in the polymeric nanofiber matrix. The UV-Vis absorption and photoluminescence spectroscopy studies indicated the quantum confinement effect of Ge-NCs on the optical properties of the electrospun Ge-NCs/PVA nanoweb. © 2013 Elsevier Ltd. All rights reserved.
Open Access
A plasmonic enhanced photodetector based on silicon nanocrystals obtained through laser ablation
(Institute of Physics Publishing, 2012-10-18) Alkis, S.; Oruç, F. B.; Ortaç, B.; Koşger, A. C.; Okyay, Ali Kemal
We present a proof-of-concept photodetector which is sensitive in the visible spectrum. Silicon nanocrystals (Si-NCs) obtained by laser ablation are used as the active absorption region. Si-NC films are formed from a polymeric dispersion. The films are sandwiched between thin insulating films to reduce the electrical leakage current. Furthermore, Ag nanoparticles are integrated with the photodetector to enhance the visible response using plasmonic effects. The measured photocurrent is resonantly enhanced, which is explained in terms of enhanced local fields caused by localized plasmons. The UV-vis spectrum of Ag nanoparticles is also measured to verify the resonance.
Open Access
Property enhancement in unsaturated polyester nanocomposites by using a reactive intercalant for clay modification
(Wiley, 2013) Şen, S.; Gündem, H. B.; Ortaç, B.
Polymeric nanocomposites were synthesized from unsaturated polyester (UPE) matrix and montmorillonite (MMT) clay using an in situ free radical polymerization reaction. Organophilic MMT was obtained using a quaternary salt of coco amine as intercalant having a styryl group making it a reactive intercalant. The resultant nanocomposites were characterized via X-ray diffraction and transmission electron microscopy. The effect of increased nanofiller loading on the thermal and mechanical properties of the nanocomposites was investigated. All the nanocomposites were found to have improved thermal and mechanical properties as compared with neat UPE matrix, resulting from the contribution of nanolayer connected intercalant-to- crosslinker which allows a crosslinking reaction. It was found that the partially exfoliated nanocomposite structure with an exfoliation dominant morphology was achieved when the MMT loading was 1 wt %. This nanocomposite exhibited the highest thermal stability, the best dynamic mechanical performance and the highest crosslinking density, most probably due to more homogeneous dispersion and optimum amount of styrene monomer molecules inside and outside the MMT layers at 1 wt % loading. Copyright © 2013 Wiley Periodicals, Inc.