Tailoring vibrational signature and functionality of 2d-ordered linear-chain carbon-based nanocarriers for predictive performance enhancement of high-end energetic materials

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buir.contributor.authorGülseren, Oğuz
buir.contributor.orcidGülseren, Oğuz|0000-0002-7632-0954
dc.citation.epage25en_US
dc.citation.issueNumber7en_US
dc.citation.spage1en_US
dc.citation.volumeNumber12en_US
dc.contributor.authorLukin, Alexander
dc.contributor.authorGülseren, Oğuz
dc.date.accessioned2023-03-02T13:19:44Z
dc.date.available2023-03-02T13:19:44Z
dc.date.issued2022-04-01
dc.departmentDepartment of Physicsen_US
dc.description.abstractA recently proposed, game-changing transformative energetics concept based on predictive synthesis and preprocessing at the nanoscale is considered as a pathway towards the development of the next generation of high-end nanoenergetic materials for future multimode solid propulsion systems and deep-space-capable small satellites. As a new door for the further performance enhancement of transformative energetic materials, we propose the predictive ion-assisted pulse-plasma-driven assembling of the various carbon-based allotropes, used as catalytic nanoadditives, by the 2D-ordered linear-chained carbon-based multicavity nanomatrices serving as functionalizing nanocarriers of multiple heteroatom clusters. The vacant functional nanocavities of the nanomatrices available for heteroatom doping, including various catalytic nanoagents, promote heat transfer enhancement within the reaction zones. We propose the innovative concept of fine-tuning the vibrational sig-natures, functionalities and nanoarchitectures of the mentioned nanocarriers by using the surface acoustic waves-assisted micro/nanomanipulation by the pulse-plasma growth zone combined with the data-driven carbon nanomaterials genome approach, which is a deep materials informatics-based toolkit belonging to the fourth scientific paradigm. For the predictive manipulation by the micro-and mesoscale, and the spatial distribution of the induction and energy release domains in the reaction zones, we propose the activation of the functionalizing nanocarriers, assembled by the heteroatom clusters, through the earlier proposed plasma-acoustic coupling-based technique, as well as by the Teslaphoresis force field, thus inducing the directed self-assembly of the mentioned nanocarbon-based additives and nanocarriers. © 2022 by the authors. Licensee MDPI, Basel, Switzerland.en_US
dc.description.provenanceSubmitted by Cem Çağatay Akgün (cem.akgun@bilkent.edu.tr) on 2023-03-02T13:19:44Z No. of bitstreams: 1 Tailoring_Vibrational_Signature_and_Functionality_of_2D-Ordered_Linear-Chain_Carbon-Based_Nanocarriers_for_Predictive_Performance_Enhancement_of_High-End_Energetic_Materials.pdf: 6121593 bytes, checksum: cdd2892bbd14ae954eef8bb095e4ca4a (MD5)en
dc.description.provenanceMade available in DSpace on 2023-03-02T13:19:44Z (GMT). No. of bitstreams: 1 Tailoring_Vibrational_Signature_and_Functionality_of_2D-Ordered_Linear-Chain_Carbon-Based_Nanocarriers_for_Predictive_Performance_Enhancement_of_High-End_Energetic_Materials.pdf: 6121593 bytes, checksum: cdd2892bbd14ae954eef8bb095e4ca4a (MD5) Previous issue date: 2022-04-01en
dc.identifier.doi10.3390/nano12071041en_US
dc.identifier.issn20794991
dc.identifier.urihttp://hdl.handle.net/11693/112026
dc.language.isoEnglishen_US
dc.publisherMDPIen_US
dc.relation.isversionofhttps://dx.doi.org/10.3390/nano12071041en_US
dc.source.titleNanomaterialsen_US
dc.subjectData-driven carbon nanomaterials genome approachen_US
dc.subjectDirected self-assemblyen_US
dc.subjectHeteroatom dopingen_US
dc.subjectIon-assisted pulse-plasma assemblingen_US
dc.subjectPlasma-acoustic coupling mechanismen_US
dc.subjectSurface acoustic wavesen_US
dc.subjectTransformative energeticsen_US
dc.subjectUnified templatesen_US
dc.subjectVibrational signatureen_US
dc.titleTailoring vibrational signature and functionality of 2d-ordered linear-chain carbon-based nanocarriers for predictive performance enhancement of high-end energetic materialsen_US
dc.typeArticleen_US

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