Efficient generation of emissive many-body correlations in copper-doped colloidal quantum wells
buir.contributor.author | Hernandez Martinez, Pedro Ludwig | |
buir.contributor.author | Delikanlı, Savaş | |
buir.contributor.author | Altintas, Yemliha | |
buir.contributor.author | Demir, Hilmi Volkan | |
buir.contributor.orcid | Hernandez Martinez, Pedro Ludwig|0000-0001-6158-0430 | |
buir.contributor.orcid | Demir, Hilmi Volkan|0000-0003-1793-112X | |
dc.citation.epage | 12 | en_US |
dc.citation.issueNumber | 9 | en_US |
dc.citation.spage | 1 | en_US |
dc.citation.volumeNumber | 3 | en_US |
dc.contributor.author | Yu, Junhong | |
dc.contributor.author | Sharma, Manoj | |
dc.contributor.author | Li, Mingjie | |
dc.contributor.author | Liu, Baiquan | |
dc.contributor.author | Hernández-Martínez, Pedro Ludwig | |
dc.contributor.author | Delikanli, Savaş | |
dc.contributor.author | Sharma, Ashma | |
dc.contributor.author | Altintas, Yemliha | |
dc.contributor.author | Hettiarachchi, Chathuranga | |
dc.contributor.author | Sum, Tze Chien | |
dc.contributor.author | Demir, Hilmi Volkan | |
dc.contributor.author | Dang, Cuong | |
dc.date.accessioned | 2023-02-27T17:36:05Z | |
dc.date.available | 2023-02-27T17:36:05Z | |
dc.date.issued | 2022-09-21 | |
dc.department | Department of Electrical and Electronics Engineering | en_US |
dc.description.abstract | Colloidal quantum wells (CQWs) provide an appealing platform to achieve emissive many-body correlations for novel optoelectronic devices, given that they act as hosts for strong carrier Coulomb interactions and present suppressed Auger recombination. However, the demonstrated high-order excitonic emission in CQWs requires ultrafast pumping with high excitation levels and can only be spectrally resolved at the single-particle level under cryogenic conditions. Here, through systematic investigation using static power-dependent emission spectroscopy and transient carrier dynamics, we show that Cu-doped CdSe CQWs exhibit continuous-wave-pumped high-order excitonic emission at room temperature with a large binding energy of ∼64 meV. We attribute this unique behavior to dopant excitons in which the ultralong lifetime and the highly localized wavefunction facilitate the formation of many-body correlations. The spectrally resolved high-order excitonic emission generated at power levels compatible with solar irradiation and electrical injection might pave the way for novel solution-processed solid-state devices. © 2022 The Authors | en_US |
dc.description.provenance | Submitted by Cem Çağatay Akgün (cem.akgun@bilkent.edu.tr) on 2023-02-27T17:36:05Z No. of bitstreams: 1 Efficient_generation_of_emissive_many-body_correlations_in_copper-doped_colloidal_quantum_wells.pdf: 3060955 bytes, checksum: 9e9cb39434622f2fece3d4f3d8c39197 (MD5) | en |
dc.description.provenance | Made available in DSpace on 2023-02-27T17:36:05Z (GMT). No. of bitstreams: 1 Efficient_generation_of_emissive_many-body_correlations_in_copper-doped_colloidal_quantum_wells.pdf: 3060955 bytes, checksum: 9e9cb39434622f2fece3d4f3d8c39197 (MD5) Previous issue date: 2022-09-21 | en |
dc.identifier.doi | 10.1016/j.xcrp.2022.101049 | en_US |
dc.identifier.issn | 26663864 | |
dc.identifier.uri | http://hdl.handle.net/11693/111850 | |
dc.language.iso | English | en_US |
dc.publisher | Cell Press | en_US |
dc.relation.isversionof | https://dx.doi.org/10.1016/j.xcrp.2022.101049 | en_US |
dc.source.title | Cell Reports Physical Science | en_US |
dc.subject | Colloidal nanocrystals | en_US |
dc.subject | Colloidal quantum wells | en_US |
dc.subject | Copper doping | en_US |
dc.subject | High-order excitonic states | en_US |
dc.subject | Ultrafast spectroscopy | en_US |
dc.title | Efficient generation of emissive many-body correlations in copper-doped colloidal quantum wells | en_US |
dc.type | Article | en_US |
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