Browsing by Subject "Whispering - gallery - mode lasing"

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    Observation of polarized gain from aligned colloidal nanorods
    (Royal Society of Chemistry, 2015) Gao, Y.; Ta, V. D.; Zhao, X.; Wang Y.; Chen R.; Mutlugün, E.; Fong, K. E.; Tan S.T.; Dang C.; Sun, X. W.; Sun, H.; Demir, Hilmi Volkan
    In recent years, colloidal semiconductor nanorods have attracted great interest for polarized spontaneous emission. However, their polarized gain has not been possible to achieve so far. In this work we show the highly polarized stimulated emission from the densely packed ensembles of core-seeded nanorods in a cylindrical cavity. Here CdSe/CdS dot-in-rods were coated and aligned on the inner wall of a capillary tube, providing optical feedback for the nanorod gain medium. Results show that the polarized gain originates intrinsically from the aligned nanorods and not from the cavity and that the optical anisotropy of the nanorod ensemble was amplified with the capillary tube, resulting in highly polarized whispering gallery mode lasing. The highly polarized emission and lasing, together with easy fabrication and flexible incorporation, make this microlaser a promising candidate for important color conversion and enrichment applications including liquid crystal display backlighting and laser lighting. This journal is © The Royal Society of Chemistry.
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    Unraveling the ultralow threshold stimulated emission from CdZnS/ZnS quantum dot and enabling high ‐ Q microlasers
    (Wiley-VCH Verlag, 2015) Wang Y.; Fong, K. E.; Yang, S.; Ta, V.; Gao, Y.; Wang, Z.; Nalla, V.; Demir, Hilmi Volkan; Sun, H.
    The newly engineered ternary CdZnS/ZnS colloidal quantum dots (CQDs) are found to exhibit remarkably high photoluminescence quantum yield and excellent optical gain properties. However, the underlying mechanisms, which could offer the guidelines for devising CQDs for optimized photonic devices, remain undisclosed. In this work, through comprehensive steady-state and time-resolved spectroscopy studies on a series of CdZnS-based CQDs, we unambiguously clarify that CdZnS-based CQDs are inherently superior optical gain media in the blue spectral range due to the slow Auger process and that the ultralow threshold stimulated emission is enabled by surface/interface engineering. Furthermore, external cavity-free high-Q quasitoroid microlasers were produced from self-assembly of CdZnS/ZnS CQDs by facile inkjet printing technique. Detailed spectroscopy analysis confirms the whispering gallery mode lasing mechanism of the quasitoroid microlasers. This tempting microlaser fabrication method should be applicable to other solution-processed gain materials, which could trigger broad research interests. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA.