Browsing by Subject "Strong coupling"
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Item Open Access Ground state energy of the fröhlich polaron as a function of dimensionality and the phonon coupling strength(2018-09) Bayrak, Hamdi BurakWe use the trial polaron wave function introduced by Devreese et al. [1] to estimate the ground state energies of the Fröhlich polaron over a broad range of the phonon coupling strength by a variational approach. We calculate the binding energy of the polaron as a function of dimensionality interpolating between two and three dimensions. We compare these results with the outcomes obtained by the Strong and Weak Coupling Theories and conclude that in the strong coupling regime, the present work leads to a significantly improved upper bound for the ground state energy.Item Open Access Lasing in a Slow Plasmon Moiré Cavity(American Chemical Society, 2015) Karademir, E.; Balci, S.; Kocabas, C.; Aydınlı, AtillaWe report on lasing from dye-based excitons coupled to slow plasmon states inside metallic Moiré cavities. Surface plasmon polaritons (SPPs) inside the cavity were slowed down to a maximum group velocity of 0.3c. Varying the modulation of the Moiré cavity, we tune the output wavelength of the plasmonic laser by varying the fast modulation period of the Moiré cavity. This work opens a new way to study SPP-matter interaction dynamics and plasmonic lasing with Bragg cavity confined slow plasmons.Item Open Access Quantum bistability, structural transformation, and spontaneous persistent currents in mesoscopic aharonov-bohm loops(World Scientific Publishing Co., 2005) Kulik, I. O.Fixed-number-of-electron mesoscopic or macromolecular conducting ring is shown to support persistent currents due to Aharonov-Bohm flux, and the "spontaneous" persistent currents without the flux when structural transformation in the ring is blocked by strong coupling to the externally azimuthal-symmetric environment. In the free-standing macromolecular ring, symmetry breaking removes the azimuthal periodicity which however is further restored at the increasing field. Three-site ring with one or three electrons represent an interesting quantum system which can serve as a qubit (quantum bit of information) and a qugate (quantum logical gate). © 2005 by World Scientific Publishing Co. Pte. Ltd.Item Open Access Raman enhancement on a broadband meta-surface(American Chemical Society, 2012-07-30) Ayas S.; Güner, H.; Türker, B.; Ekiz, O. O.; Dirisaglik, F.; Okyay, Ali Kemal; Dâna, A.Plasmonic metamaterials allow confinement of light to deep subwavelength dimensions, while allowing for the tailoring of dispersion and electromagnetic mode density to enhance specific photonic properties. Optical resonances of plasmonic molecules have been extensively investigated; however, benefits of strong coupling of dimers have been overlooked. Here, we construct a plasmonic meta-surface through coupling of diatomic plasmonic molecules which contain a heavy and light meta-atom. Presence and coupling of two distinct types of localized modes in the plasmonic molecule allow formation and engineering of a rich band structure in a seemingly simple and common geometry, resulting in a broadband and quasi-omni-directional meta-surface. Surface-enhanced Raman scattering benefits from the simultaneous presence of plasmonic resonances at the excitation and scattering frequencies, and by proper design of the band structure to satisfy this condition, highly repeatable and spatially uniform Raman enhancement is demonstrated. On the basis of calculations of the field enhancement distribution within a unit cell, spatial uniformity of the enhancement at the nanoscale is discussed. Raman scattering constitutes an example of nonlinear optical processes, where the wavelength conversion during scattering may be viewed as a photonic transition between the bands of the meta-material.Item Open Access Strong coupling between localized and propagating plasmon polaritons(OSA - The Optical Society, 2015) Balci, S.; Karademir, E.; Kocabas, C.We investigate plasmon-plasmon (PP) coupling in the strongly interacting regimes by using a tunable plasmonic platform consisting of triangular Ag nanoprisms placed nanometers away from Ag thin films. The nanoprisms are colloidally synthesized using a seed-mediated growth method and having size-tunable localized surface plasmon polariton (SPP) resonances immobilized on Si3N4 films. The PP coupling between the localized SPPs of metal nanoprisms and the propagating SPPs of the metal film is controlled by the nanoprism concentration and the plasmon damping in the metal film. Results reveal that Rabi splitting energy determining the strength of the coupling can reach up to several hundreds meV, thus demonstrating the ultrastrong coupling occurring between localized and propagating SPPs. The metal nanoparticle-metal thin film hybrid system over the square-centimeter areas presented here provides a unique configuration to study PP coupling all the way from the weak to ultrastrong coupling regimes in a broad range of wavelengths.Item Open Access Tunable plexcitonic nanoparticles: a model system for studying plasmon-exciton interaction from the weak to the ultrastrong coupling regime(American Chemical Society, 2016) Balci, S.; Kucukoz, B.; Balci, O.; Karatay, A.; Kocabas, C.; Yaglioglu, G.Controlling the number of dye molecules on metallic nanoparticles, which in turn affects the magnitude of Rabi splitting energy, is crucial for obtaining hybrid metal core–organic shell nanoparticles with tunable optical properties in the visible spectrum since the magnitude of the Rabi splitting energy directly determines the strength of the coupling between plasmonic nanoparticles and dye molecules. In this work, we present a new method for the synthesis of plexcitonic nanoparticles, and thus we are able to control the number of dye molecules self-assembled on Ag nanoprisms (Ag NPs) by adjusting the concentration of dye molecules used in the synthesis. Indeed, individual dye molecules self-assemble into J-aggregates on Ag NPs. Thus, in the finite-element simulations and experimental data of the hybrid metal organic nanoparticles, we observed a transition from weak coupling to the ultrastrong coupling regime. Besides, ultrafast energy transfer between plasmonic nanoparticles and excitonic aggregated dye molecules has been extensively studied as a function of Rabi splitting energy. We observe that the lifetime of the polariton states increases with the coupling strength and the upper polaritons are short-lived, whereas the lower polaritons are long-lived. Hybrid metal–organic nanoparticles presented in this study (i) have tunable Rabi splitting energies, (ii) are easy to prepare in large quantities in aqueous medium, (iii) can be uniformly assembled on solid substrates, (iv) have resonance frequencies in the visible spectrum, and (v) have small mode volume, thus making them an excellent model system for studying light–matter interaction at nanoscale dimensions from the weak to ultrastrong coupling regime.