Browsing by Subject "Mie resonance"

Now showing 1 - 4 of 4

Open Access
Lasing action in single subwavelength particles supporting supercavity modes
(American Chemical Society, 2020-05) Mylnikov, V.; Ha, S. T.; Pan, Z.; Valuckas, V.; Paniagua-Domínguez, R.; Demir, Hilmi Volkan; Kuznetsov, A. I.
On-chip light sources are critical for the realization of fully integrated photonic circuitry. So far, semiconductor miniaturized lasers have been mainly limited to sizes on the order of a few microns. Further reduction of sizes is challenging fundamentally due to the associated radiative losses. While using plasmonic metals helps to reduce radiative losses and sizes, they also introduce Ohmic losses hindering real improvements. In this work, we show that, making use of quasibound states in the continuum, or supercavity modes, we circumvent these fundamental issues and realize one of the smallest purely semiconductor nanolasers thus far. Here, the nanolaser structure is based on a single semiconductor nanocylinder that intentionally takes advantage of the destructive interference between two supported optical modes, namely Fabry–Perot and Mie modes, to obtain a significant enhancement in the quality factor of the cavity. We experimentally demonstrate the concept and obtain optically pumped lasing action using GaAs at cryogenic temperatures. The optimal nanocylinder size is as small as 500 nm in diameter and only 330 nm in height with a lasing wavelength around 825 nm, corresponding to a size-to-wavelength ratio as low as 0.6.
Open Access
Polariton lasing in Mie-resonant perovskite nanocavity
(Editorial Office of Opto-Electronic Advances, 2024-01-19) Masharin, Mikhail A.; Khmelevskaia, Daria; Kondratiev, Valeriy I.; Markina, Daria I.; Utyushev, Anton D.; Dolgintsev, Dmitriy M.; Dmitriev, Alexey D.; Shahnazaryan, Vanik A.; Pushkarev, Anatoly P.; Işık, Furkan; Iorsh, Ivan V.; Shelykh, Ivan A.; Demir, Hilmi Volkan; Samusev, Anton K.; Makarov, Sergey V.
Deeply subwavelength lasers (or nanolasers) are highly demanded for compact on-chip bioimaging and sensing at the nanoscale. One of the main obstacles for the development of single-particle nanolasers with all three dimensions shorter than the emitting wavelength in the visible range is the high lasing thresholds and the resulting overheating. Here we exploit exciton-polariton condensation and mirror-image Mie modes in a cuboid CsPbBr₃ nanoparticle to achieve coherent emission at the visible wavelength of around 0.53 μm from its ultra-small (≈0.007 μm³ or ≈λ³/20) semiconductor nanocavity. The polaritonic nature of the emission from the nanocavity localized in all three dimensions is proven by direct comparison with corresponding one-dimensional and two-dimensional waveguiding systems with similar material parameters. Such a deeply subwavelength nanolaser is enabled not only by the high values for exciton binding energy (≈35 meV), refractive index (>2.5 at low temperature), and luminescence quantum yield of CsPbBr₃, but also by the optimization of polaritons condensation on the Mie resonances with quality factors improved by the metallic substrate. Moreover, the key parameters for optimal lasing conditions are intermode free spectral range and phonons spectrum in CsPbBr₃, which govern polaritons condensation path. Such chemically synthesized colloidal CsPbBr₃ nanolasers can be potentially deposited on arbitrary surfaces, which makes them a versatile tool for integration with various on-chip systems.
Open Access
A simple mie-resonator based meta-array with diverse deflection scenarios enabling multifunctional operation at near-infrared
(De Gruyter Open, 2020) Aalizadeh, Majid; Serebryannikov, A. E.; Özbay, Ekmel; Vandenbosch, G. A. E.
Deflection, a basic functionality of wavefront manipulation is usually associated with the phase-gradient metasurfaces and the classical blazed gratings. We numerically and experimentally demonstrate an unusually wideband and simultaneously wide-angle deflection achieved at near-infrared in reflection mode for a periodic (nongradient), ultrathin meta-array comprising only one silicon nanorod (Mie resonator) per period. It occurs in the range where only the first negative diffraction order and zero order may propagate. Deflection serves as the enabler for multifunctional operation. Being designed with the main goal to obtain ultra-wideband and wide-angle deflection, the proposed meta-array is also capable in spatial filtering and wide-angle splitting. Spatial filtering of various types can be obtained in one structure by exploiting either deflection in nonzero diffraction orders, or the specular-reflection (zero-order) regime. Thus, the role of different diffraction orders is clarified. Moreover, on–off switching of deflection and related functionalities is possible by changing polarization state of the incident wave. The suggested device is simple to fabricate and only requires cost-effective materials, so it is particularly appropriate for the large-area fabrication using nanoprint lithography. Ultra-wideband wide-angle and other deflection scenarios, along with the other functionalities, are promising for applications in optical communications, laser optics, sensing, detection, and imaging.
Open Access
Subwavelength densely packed disordered semiconductor metasurface units for photoelectrochemical hydrogen generation
(American Chemical Society, 2022-03-10) Ulusoy Ghobadi, T. Gamze; Ghobadi, Amir; Odabaşı, Oğuz; Karadaş, Ferdi; Özbay, Ekmel
For most semiconductors, especially the visible-light-absorbing ones, the carrier diffusion length is significantly shorter than the light penetration depth, limiting their photoactivities. This limitation could be mitigated through the use of subwavelength semiconductor-based metasurfaces and metamaterials. In this paper, a large-scale compatible metasurface photocathode, made of densely packed disordered p-type chromium oxide (CrOX), is developed to be utilized in photoelectrochemical (PEC) hydrogen generation. For this purpose, first, tightly packed random Cr nanorods are fabricated using an oblique angle deposition technique. Afterward, an annealing step is applied to the sample to transform these metallic units into a semiconducting p-type CrOX-based metasurface. Based on the experimental characterization results and numerical simulations, the proposed design can provide strong light-matter interactions in an ultra-broadband-wavelength range, mainly due to its multidimensional random geometry and ultrasmall gap sizes. Finally, to substantiate the activity of the CrOXnanorods, a core-crown geometry is developed where the NiOXcapping layer catalyzes the hydrogen evolution reaction (HER). The proposed heterostructure metasurface absorber can impose photocurrent values as large as 50 μA cm-2with a photocurrent spectral response extended up to 500 nm. Moreover, the electrode shows outstanding operation under light irradiation for 9 hours. This work demonstrates a simple, scalable design strategy to fabricate low-cost and stable photocathodes for PEC hydrogen evolution. © 2022 American Chemical Society. All rights reserved.