Browsing by Author "Küçüköz, B."

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    Probing ultrafast energy transfer between excitons and plasmons in the ultrastrong coupling regime
    (American Institute of Physics Inc., 2014) Balci, S.; Kocabas, C.; Küçüköz, B.; Karatay, A.; Akhüseyin, E.; Yaglioglu, H. G.; Elmali, A.
    We investigate ultrafast energy transfer between excitons and plasmons in ensembles of core-shell type nanoparticles consisting of metal core covered with a concentric thin J-aggregate (JA) shell. The high electric field localization by the Ag nanoprisms and the high oscillator strength of the JAs allow us to probe this interaction in the ultrastrong plasmon-exciton coupling regime. Linear and nonlinear optical properties of the coupled system have been measured using transient absorption spectroscopy revealing that the hybrid system shows half-plasmonic and half-excitonic properties. The tunability of the nanoprism plasmon resonance provides a flexible platform to study the dynamics of the hybrid state in a broad range of wavelengths. © 2014 AIP Publishing LLC.