Regulating the solvation structure of potassium Ions using a multidentate ether in potassium metal batteries

buir.contributor.authorÜlgüt, Burak
buir.contributor.orcidÜlgüt, Burak|0000-0002-4402-0033
dc.citation.epage10374en_US
dc.citation.issueNumber9en_US
dc.citation.spage10366en_US
dc.citation.volumeNumber5en_US
dc.contributor.authorChen, C.
dc.contributor.authorZhou, J.
dc.contributor.authorWenbinb, F.
dc.contributor.authorXueyinga, M.
dc.contributor.authorChen, S.
dc.contributor.authorSun, L.
dc.contributor.authorMeng, Y.
dc.contributor.authorTao, K.
dc.contributor.authorÜlgüt, Burak
dc.contributor.authorSun, P.
dc.contributor.authorBielawski, C.
dc.contributor.authorBielawski, C. W.
dc.contributor.authorGeng, J.
dc.date.accessioned2023-02-21T06:05:22Z
dc.date.available2023-02-21T06:05:22Z
dc.date.issued2022-09-26
dc.description.abstractPotassium (K) is regarded as an alternative to lithium (Li) for use in contemporary energy storage devices owing to its high abundance and low electrochemical potential. However, because K ions are larger than Li ions, they exhibit different solvation properties that can ultimately affect device performance. Herein, a multidentate ether-based electrolyte is demonstrated to effectively solvate K ions and the solvation structures can be further modulated with cosolvents. The use of the multidentate ether-based electrolyte also suppresses the formation of K dendrites and significantly enhances the cycling stability of K//K symmetric cells (e.g., over 2000 h at 0.25 mA cm-2). © 2022 American Chemical Society. All rights reserved.en_US
dc.identifier.doi10.1021/acsaem.2c01504en_US
dc.identifier.eissn2574-0962
dc.identifier.urihttp://hdl.handle.net/11693/111555
dc.language.isoEnglishen_US
dc.publisherAmerican Chemical Societyen_US
dc.relation.isversionofhttps://dx.doi.org/10.1021/acsaem.2c01504en_US
dc.source.titleACS Applied Energy Materialsen_US
dc.subjectDendrite-free metal anodeen_US
dc.subjectEther-based electrolytesen_US
dc.subjectMultidentate solventsen_US
dc.subjectPotassium metal anodeen_US
dc.subjectSolvation structuresen_US
dc.titleRegulating the solvation structure of potassium Ions using a multidentate ether in potassium metal batteriesen_US
dc.typeArticleen_US
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