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      Tailoring vibrational signature and functionality of 2d-ordered linear-chain carbon-based nanocarriers for predictive performance enhancement of high-end energetic materials

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      Author(s)
      Lukin, Alexander
      Gülseren, Oğuz
      Date
      2022-04-01
      Source Title
      Nanomaterials
      Print ISSN
      20794991
      Publisher
      MDPI
      Volume
      12
      Issue
      7
      Pages
      1 - 25
      Language
      English
      Type
      Article
      Item Usage Stats
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      Abstract
      A recently proposed, game-changing transformative energetics concept based on predictive synthesis and preprocessing at the nanoscale is considered as a pathway towards the development of the next generation of high-end nanoenergetic materials for future multimode solid propulsion systems and deep-space-capable small satellites. As a new door for the further performance enhancement of transformative energetic materials, we propose the predictive ion-assisted pulse-plasma-driven assembling of the various carbon-based allotropes, used as catalytic nanoadditives, by the 2D-ordered linear-chained carbon-based multicavity nanomatrices serving as functionalizing nanocarriers of multiple heteroatom clusters. The vacant functional nanocavities of the nanomatrices available for heteroatom doping, including various catalytic nanoagents, promote heat transfer enhancement within the reaction zones. We propose the innovative concept of fine-tuning the vibrational sig-natures, functionalities and nanoarchitectures of the mentioned nanocarriers by using the surface acoustic waves-assisted micro/nanomanipulation by the pulse-plasma growth zone combined with the data-driven carbon nanomaterials genome approach, which is a deep materials informatics-based toolkit belonging to the fourth scientific paradigm. For the predictive manipulation by the micro-and mesoscale, and the spatial distribution of the induction and energy release domains in the reaction zones, we propose the activation of the functionalizing nanocarriers, assembled by the heteroatom clusters, through the earlier proposed plasma-acoustic coupling-based technique, as well as by the Teslaphoresis force field, thus inducing the directed self-assembly of the mentioned nanocarbon-based additives and nanocarriers. © 2022 by the authors. Licensee MDPI, Basel, Switzerland.
      Keywords
      Data-driven carbon nanomaterials genome approach
      Directed self-assembly
      Heteroatom doping
      Ion-assisted pulse-plasma assembling
      Plasma-acoustic coupling mechanism
      Surface acoustic waves
      Transformative energetics
      Unified templates
      Vibrational signature
      Permalink
      http://hdl.handle.net/11693/112026
      Published Version (Please cite this version)
      https://dx.doi.org/10.3390/nano12071041
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      • Department of Physics 2550
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